Szegedy et al. 2013 discovered that neural network classifiers could be fooled by imperceptible input modifications, a finding they called "intriguing properties of neural networks." Goodfellow, Shlens, and Szegedy followed in 2014 with an explanation and the first systematic method for generating these modifications: the Fast Gradient Sign Method.
Standard training uses backpropagation to compute how the loss changes with respect to the model's weights, then updates the weights to reduce the loss. FGSM applies the same gradient computation differently: compute how the loss changes with respect to the input pixels (not the weights), then increase the loss by stepping in the direction the gradient points.